Episode list & details from:  TVmaze • 
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TV.com

                            Original
  Episode #     Prod #      Air Date   Titles
_____ ______ ___________  ___________ ___________________________________________

Season 1

1.     1-1                 07 Jan 61   Hot Snow
2.     1-2                 14 Jan 61   Brought to Book
3.     1-3                 21 Jan 61   Square Root of Evil
4.     1-4                 28 Jan 61   Nightmare
5.     1-5                 04 Feb 61   Crescent Moon
6.     1-6                 11 Feb 61   Girl on the Trapeze
7.     1-7                 18 Feb 61   Diamond Cut Diamond
8.     1-8                 25 Feb 61   The Radioactive Man
9.     1-9                 04 Mar 61   Ashes of Roses
10.    1-10                18 Mar 61   Hunt the Man Down
11.    1-11                01 Apr 61   Please Don't Feed the Animals
12.    1-12                15 Apr 61   Dance with Death
13.    1-13                29 Apr 61   One for the Mortuary
14.    1-14                13 May 61   The Springers
15.    1-15                27 May 61   The Frighteners
16.    1-16                10 Jun 61   The Yellow Needle
17.    1-17                24 Jun 61   Death on the Slipway
18.    1-18                08 Jul 61   Double Danger
19.    1-19                22 Jul 61   Toy Trap
20.    1-20                05 Aug 61   The Tunnel of Fear
21.    1-21                19 Aug 61   The Far Distant Dead
22.    1-22                02 Sep 61   Kill the King
23.    1-23                09 Dec 61   Dead of Winter
24.    1-24                16 Dec 61   The Deadly Air
25.    1-25                23 Dec 61   A Change of Bait
26.    1-26                30 Dec 61   Dragonsfield

Season 2

27.    2-1                 29 Sep 62   Mr Teddy Bear
28.    2-2                 06 Oct 62   Propellant 23
29.    2-3                 13 Oct 62   The Decapod
30.    2-4                 20 Oct 62   Bullseye
31.    2-5                 27 Oct 62   Mission to Montreal
32.    2-6                 03 Nov 62   The Removal Men
33.    2-7                 10 Nov 62   The Mauritius Penny
34.    2-8                 17 Nov 62   Death of a Great Dane
35.    2-9                 24 Nov 62   The Sell-Out
36.    2-10                01 Dec 62   Death on the Rocks
37.    2-11                08 Dec 62   Traitor in Zebra
38.    2-12                15 Dec 62   The Big Thinker
39.    2-13                22 Dec 62   Death Dispatch
40.    2-14                29 Dec 62   Dead on Course
41.    2-15                05 Jan 63   Intercrime
42.    2-16                12 Jan 63   Immortal Clay
43.    2-17                19 Jan 63   Box of Tricks
44.    2-18                26 Jan 63   Warlock
45.    2-19                02 Feb 63   The Golden Eggs
46.    2-20                09 Feb 63   School for Traitors
47.    2-21                16 Feb 63   The White Dwarf
48.    2-22                23 Feb 63   The Man in the Mirror
49.    2-23                02 Mar 63   Conspiracy of Silence
50.    2-24                09 Mar 63   A Chorus of Frogs
51.    2-25                16 Mar 63   Six Hands Across a Table
52.    2-26                23 Mar 63   Killer Whale

Season 3

53.    3-1                 28 Sep 63   Brief for Murder
54.    3-2                 05 Oct 63   The Undertakers
55.    3-3                 12 Oct 63   Man with Two Shadows
56.    3-4                 19 Oct 63   The Nutshell
57.    3-5                 26 Oct 63   Death of a Batman
58.    3-6                 02 Nov 63   November Five
59.    3-7                 09 Nov 63   The Gilded Cage
60.    3-8                 16 Nov 63   Second Sight
61.    3-9                 23 Nov 63   The Medicine Men
62.    3-10                30 Nov 63   The Grandeur That Was Rome
63.    3-11                07 Dec 63   The Golden Fleece
64.    3-12                14 Dec 63   Don't Look Behind You
65.    3-13                21 Dec 63   Death A La Carte
66.    3-14                28 Dec 63   Dressed to Kill
67.    3-15                04 Jan 64   The White Elephant
68.    3-16                11 Jan 64   The Little Wonders
69.    3-17                18 Jan 64   The Wringer
70.    3-18                25 Jan 64   Mandrake
71.    3-19                01 Feb 64   The Secrets Broker
72.    3-20                08 Feb 64   Trojan Horse
73.    3-21                15 Feb 64   Build a Better Mousetrap
74.    3-22                22 Feb 64   The Outside-In Man
75.    3-23                29 Feb 64   The Charmers
76.    3-24                07 Mar 64   Concerto
77.    3-25                14 Mar 64   Esprit De Corps
78.    3-26                21 Mar 64   Lobster Quadrille

Season 4

79.    4-1                 02 Oct 65   The Town of No Return
80.    4-2                 09 Oct 65   The Gravediggers
81.    4-3                 16 Oct 65   The Cybernauts
82.    4-4                 23 Oct 65   Death at Bargain Prices
83.    4-5                 30 Oct 65   Castle De'ath
84.    4-6                 06 Nov 65   The Master Minds
85.    4-7                 13 Nov 65   The Murder Market
86.    4-8                 20 Nov 65   A Surfeit of H2O
87.    4-9                 27 Nov 65   The Hour that Never Was
88.    4-10                04 Dec 65   Dial a Deadly Number
89.    4-11                11 Dec 65   Man-Eater of Surrey Green
90.    4-12                18 Dec 65   Two's a Crowd
91.    4-13                25 Dec 65   Too Many Christmas Trees
92.    4-14                01 Jan 66   Silent Dust
93.    4-15                08 Jan 66   Room Without a View
94.    4-16                15 Jan 66   Small Game For Big Hunters
95.    4-17                22 Jan 66   The Girl From Auntie
96.    4-18                29 Jan 66   The Thirteenth Hole
97.    4-19                05 Feb 66   Quick-Quick Slow Death
98.    4-20                12 Feb 66   The Danger Makers
99.    4-21                19 Feb 66   A Touch of Brimstone
100.   4-22                26 Feb 66   What the Butler Saw
101.   4-23                05 Mar 66   The House That Jack Built
102.   4-24                12 Mar 66   A Sense of History
103.   4-25                19 Mar 66   How to Succeed... at Murder
104.   4-26                26 Mar 66   Honey For the Prince

Season 5

105.   5-1                 14 Jan 67   From Venus With Love
106.   5-2                 21 Jan 67   The Fear Merchants
107.   5-3                 28 Jan 67   Escape in Time
108.   5-4                 04 Feb 67   The See-Through Man
109.   5-5                 11 Feb 67   The Bird Who Knew Too Much
110.   5-6                 18 Feb 67   The Winged Avenger
111.   5-7                 25 Feb 67   The Living Dead
112.   5-8                 04 Mar 67   The Hidden Tiger
113.   5-9                 11 Mar 67   The Correct Way to Kill
114.   5-10                18 Mar 67   Never, Never Say Die
115.   5-11                01 Apr 67   Epic
116.   5-12                08 Apr 67   The Superlative Seven
117.   5-13                15 Apr 67   A Funny Thing Happened on the Way to the Station
118.   5-14                22 Apr 67   Something Nasty in the Nursery
119.   5-15                29 Apr 67   The Joker
120.   5-16                06 May 67   Who's Who???
121.   5-17                30 Sep 67   Return of the Cybernauts
122.   5-18                07 Oct 67   Death's Door
123.   5-19                14 Oct 67   The 50,000 Pound Breakfast
124.   5-20                21 Oct 67   Dead Man's Treasure
125.   5-21                28 Oct 67   You Have Just Been Murdered
126.   5-22                04 Nov 67   The Positive Negative Man
127.   5-23                11 Nov 67   Murdersville
128.   5-24                18 Nov 67   Mission... Highly Improbable

Season 6

129.   6-1                 25 Sep 68   The Forget-Me-Knot
130.   6-2                 02 Oct 68   Game
131.   6-3                 09 Oct 68   Super Secret Cypher Snatch
132.   6-4                 16 Oct 68   You'll Catch Your Death
133.   6-5                 23 Oct 68   Split!
134.   6-6                 30 Oct 68   Whoever Shot Poor George Oblique Stroke XR40
135.   6-7                 06 Nov 68   False Witness
136.   6-8                 13 Nov 68   All Done With Mirrors
137.   6-9                 20 Nov 68   Legacy of Death
138.   6-10                27 Nov 68   Noon Doomsday
139.   6-11                04 Dec 68   Look- (stop me if you've heard this one) But There Were These Two Fellers...
140.   6-12                11 Dec 68   Have Guns- Will Haggle
141.   6-13                18 Dec 68   They Keep Killing Steed
142.   6-14                01 Jan 69   The Interrogators
143.   6-15                08 Jan 69   The Rotters
144.   6-16                15 Jan 69   Invasion of the Earthmen
145.   6-17                22 Jan 69   Killer
146.   6-18                29 Jan 69   The Morning After
147.   6-19                05 Feb 69   The Curious Case of the Countless Clues
148.   6-20                12 Feb 69   Wish You Were Here
149.   6-21                19 Feb 69   Love All
150.   6-22                26 Feb 69   Stay Tuned
151.   6-23                05 Mar 69   Take Me To Your Leader
152.   6-24                12 Mar 69   Fog
153.   6-25                19 Mar 69   Who Was That Man I Saw You With?
154.   6-26                26 Mar 69   Homicide And Old Lace
155.   6-27                02 Apr 69   Thingumajig
156.   6-28                07 Apr 69   My Wildest Dream
157.   6-29                16 Apr 69   Requiem
158.   6-30                23 Apr 69   Take-Over
159.   6-31                30 Apr 69   Pandora
160.   6-32                14 May 69   Get-A-Way
161.   6-33                21 May 69   Bizarre


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